dorsal/arxiv
View SchemaMagnetic field-induced phases in a model S=1 Haldane chain system
| Authors | I. Jakovac, M. S. Grbić, M. Dupont, N. Laflorencie, S. Capponi, Y. Hosokoshi, S. Krämer, Y. Skourski, S. Luther M. Takigawa, M. Horvatić |
|---|---|
| Categories | |
| ArXiv ID | 2601.10489vv1 |
| URL | https://arxiv.org/abs/2601.10489 |
| License | http://arxiv.org/licenses/nonexclusive-distrib/1.0/ |
Abstract
An $S=1$ Haldane chain is a one-dimensional (1D) quantum magnet where strong fluctuations result in quantum disordered singlet ground state with a gapped excitation spectrum. The gap magnitude is primarily set by the dominant intrachain interaction ($J_\text{1D}$). An applied magnetic field closes the gap at $B_\text{c1}$ and drives the system into a gapless Tomonaga-Luttinger liquid (TLL) regime, followed by, at lower temperatures, a Bose-Einstein condensate (BEC) ground state, persisting up to $B_\text{c2} \propto 4 J_\text{1D}/g\mu_B$. Almost all previously studied experimental realizations of such systems were based on transition-metal complexes which typically suffer from intrinsic anisotropies or large $J_\text{1D}$ values, limiting the access to the full theoretical phase diagram. We report a comprehensive study of TLL and BEC phases in the organic Haldane chain system 3,5-bis(N-tert-butylaminoxyl)-3'-nitrobiphenyl (BoNO). The absence of anisotropy and a moderate $J_\text{1D}$ enable exploration of the complete $B-T$ phase diagram. Through $^1$H nuclear magnetic resonance, combined with theoretical analysis, we characterize the TLL properties, map the BEC phase boundary $T_c (B)$, determine the associated critical exponent $\nu \approx 0.66$ at $B_\text{c2}$, and demonstrate universal quasiparticle scaling in the quantum-critical regime. These results provide full experimental validation of theoretical predictions for field-induced phases in an $S=1$ Haldane chain, made over two decades ago.
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"abstract": "An $S=1$ Haldane chain is a one-dimensional (1D) quantum magnet where strong fluctuations result in quantum disordered singlet ground state with a gapped excitation spectrum. The gap magnitude is primarily set by the dominant intrachain interaction ($J_\\text{1D}$). An applied magnetic field closes the gap at $B_\\text{c1}$ and drives the system into a gapless Tomonaga-Luttinger liquid (TLL) regime, followed by, at lower temperatures, a Bose-Einstein condensate (BEC) ground state, persisting up to $B_\\text{c2} \\propto 4 J_\\text{1D}/g\\mu_B$. Almost all previously studied experimental realizations of such systems were based on transition-metal complexes which typically suffer from intrinsic anisotropies or large $J_\\text{1D}$ values, limiting the access to the full theoretical phase diagram. We report a comprehensive study of TLL and BEC phases in the organic Haldane chain system 3,5-bis(N-tert-butylaminoxyl)-3\u0027-nitrobiphenyl (BoNO). The absence of anisotropy and a moderate $J_\\text{1D}$ enable exploration of the complete $B-T$ phase diagram. Through $^1$H nuclear magnetic resonance, combined with theoretical analysis, we characterize the TLL properties, map the BEC phase boundary $T_c (B)$, determine the associated critical exponent $\\nu \\approx 0.66$ at $B_\\text{c2}$, and demonstrate universal quasiparticle scaling in the quantum-critical regime. These results provide full experimental validation of theoretical predictions for field-induced phases in an $S=1$ Haldane chain, made over two decades ago.",
"arxiv_id": "2601.10489",
"authors": [
"I. Jakovac",
"M. S. Grbi\u0107",
"M. Dupont",
"N. Laflorencie",
"S. Capponi",
"Y. Hosokoshi",
"S. Kr\u00e4mer",
"Y. Skourski",
"S. Luther M. Takigawa",
"M. Horvati\u0107"
],
"categories": [
"cond-mat.str-el"
],
"license": "http://arxiv.org/licenses/nonexclusive-distrib/1.0/",
"title": "Magnetic field-induced phases in a model S=1 Haldane chain system",
"url": "https://arxiv.org/abs/2601.10489",
"version": "v1"
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"variant": "snapshot-2026-01-17",
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